Magnetization-polarization cross-control near room temperature in hexaferrite single crystals

In their publication “Magnetization-polarization cross-control near room temperature in hexaferrite single crystals” V. Kocsis, T. Nakajima, M. Matsuda, A. Kikkawa, Y. Kaneko, J. Takashima, K. Kakurai, T. Arima, F. Kagawa, Y. Tokunaga, Y. Tokura and Y. Taguchi report that they have successfully stabilized a simultaneously ferrimagnetic and ferroelectric phase in a Y-type hexaferrite single crystal up to 450 K, and demonstrated the reversal of large non-volatile M by E field close to room temperature. Manipulation of the magnetic domains by E field was directly visualized at room temperature by using magnetic force microscopy.*

NanoWorld MFMR AFM probes with a hard magnetic coating were used for the magnetic force microscopy measurements described in this article.

Figure 5 from “Magnetization-polarization cross-control near room temperature in hexaferrite single crystals” by V. Kocsis et al.: Real-space magnetic force microscopy (MFM) images. The MFM images were taken on the same 10 × 10 μm2 region of a BSCFAO crystal with an ac face (see Supplementary Figs. 3, 9 and 10) at room temperature. Prior to the MFM measurements, the sample was poled to a single-domain ME state using (+E0, +H0) poling fields in a E ⊥ H; E, H ⊥ c configuration. Panel a shows the changes in the magnetic domain pattern caused by two successive applications of the E field with different signs (the initial state is labeled as the 0th). The images include small regions, R1 and R2, where two representative cases of DW motion are observed. Around R1, the negatively magnetized domain (denoted with blue color, MFM phase shift Δφ < 0) expands and shrinks along the c-axis upon the first and second applications of E-field, respectively. On the other hand, around R2, a positively magnetized domain (denoted with red color, Δφ > 0) is pushed into the view area from the upper side along the ab plane. These two cases are further displayed as line profiles of the MFM phase shift (Δφ) data along the b A−A′ and c B−B′ lines. Panels d, e show the schematic illustration of these two cases of domain wall motions for the second E-field switch, respectively. NanoWorld MFMR AFM probes were used for the magnetic force microscopy.
Figure 5 from “Magnetization-polarization cross-control near room temperature in hexaferrite single crystals” by V. Kocsis et al.: Real-space magnetic force microscopy (MFM) images. The MFM images were taken on the same 10 × 10 μm2 region of a BSCFAO crystal with an ac face (see Supplementary Figs. 3, 9 and 10) at room temperature. Prior to the MFM measurements, the sample was poled to a single-domain ME state using (+E0, +H0) poling fields in a E ⊥ H; E, H ⊥ c configuration. Panel a shows the changes in the magnetic domain pattern caused by two successive applications of the E field with different signs (the initial state is labeled as the 0th). The images include small regions, R1 and R2, where two representative cases of DW motion are observed. Around R1, the negatively magnetized domain (denoted with blue color, MFM phase shift Δφ < 0) expands and shrinks along the c-axis upon the first and second applications of E-field, respectively. On the other hand, around R2, a positively magnetized domain (denoted with red color, Δφ > 0) is pushed into the view area from the upper side along the ab plane. These two cases are further displayed as line profiles of the MFM phase shift (Δφ) data along the b A−A′ and c B−B′ lines. Panels d, e show the schematic illustration of these two cases of domain wall motions for the second E-field switch, respectively.

*V. Kocsis, T. Nakajima, M. Matsuda, A. Kikkawa, Y. Kaneko, J. Takashima, K. Kakurai, T. Arima, F. Kagawa, Y. Tokunaga, Y. Tokura, Y. Taguchi
Magnetization-polarization cross-control near room temperature in hexaferrite single crystals
Nature Communications, volume 10, Article number: 1247 (2019)
DOI: https://doi.org/10.1038/s41467-019-09205-x

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